Copyright (c) 2014 AJC
This work is licensed under a Creative Commons Attribution 4.0 International License.
Determination of Natural Radioactivity Levels of Some Concretes and Mineral Admixtures in Turkey
Corresponding Author(s) : Hasan Baltas
Asian Journal of Chemistry,
Vol. 26 No. 13 (2014): Vol 26 Issue 13
Abstract
Nine concrete samples with or without mineral admixtures have been analyzed for their naturally occurring radionuclide of 226Ra, 232Th and 40K using HPGe gamma spectrometry. Also, concrete raw materials such as aggregate, cement, fly ash and blast furnace slag have been measured. The radioactivity values of 226Ra, 232Th and 40K in fly ash and those of 226Ra in blast furnace slag are higher than the corresponding world mean specific activities values which are 50, 50 and 500 Bq kg-1 for 226Ra, 232Th and 40K, respectively. The concretes activity concentrations have been found to change with supplementary cementitious materials of the concrete samples. This may be attributed to containing different proportions of different mineral additives such as fly ash and blast furnace slag which were found to contain high natural radionuclide concentrations according to the rest of raw material samples. In addition, radium equivalent activities (Raeq), g-index (Ig), a-index (Ia), absorbed dose rate in air (D) and annual effective dose associated with the natural radionuclide were calculated to assess the radiation hazard of the natural radioactivity in the concrete mixture samples. The concentration of the natural radionuclides and the radium equivalent activity obtained in the present study are compared with the previous results. From these results, it can be seen that these building materials do not pose significant radiation hazards.
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- E. Yilmaz, H. Baltas, E. Kiris, İ. Ustabas, U. Cevik and A.M. El-Khayatt, Ann. Nucl. Energy, 38, 2204 (2011); doi:10.1016/j.anucene.2011.06.011.
- V. Kumar, T.V. Ramachandran and R. Prasad, Appl. Radiat. Isot., 51, 93 (1999); doi:10.1016/S0969-8043(98)00154-7.
- O. Baykara, Ş. Karatepe and M. Doğru, Radiat. Meas., 46, 153 (2011); doi:10.1016/j.radmeas.2010.08.010.
- N. Kovler, G. Haquin, V. Manasherov, E. Ne’eman and N. Lavi, Build. Environ., 37, 531 (2002); doi:10.1016/S0360-1323(01)00048-8.
- S. Stoulos, M. Manolopoulou and C. Papastefanou, J. Environ. Radioact., 69, 225 (2003); doi:10.1016/S0265-931X(03)00081-X.
- B. Mavi and I. Akkurt, Radiat. Phys. Chem., 79, 933 (2010); doi:10.1016/j.radphyschem.2010.03.019.
- H. Papaefthymiou and O. Gouseti, Radiat. Meas., 43, 1453 (2008); doi:10.1016/j.radmeas.2008.03.032.
- R. Hewamanna, C.S. Sumithrarachchi, P. Mahawatte, H.L.C. Nanayakkara and H.C. Ratnayake, Appl. Radiat. Isot., 54, 365 (2001); doi:10.1016/S0969-8043(00)00107-X.
- N.P. Petropoulos, M.J. Anagnostakis and S.E. Simopoulos, J. Environ. Radioact., 61, 257 (2002); doi:10.1016/S0265-931X(01)00132-1.
- X. Lu, G. Yang and C. Ren, Radiat. Phys. Chem., 81, 780 (2012); doi:10.1016/j.radphyschem.2012.02.043.
- U. Cevik, N. Damla, A.I. Kobya, A. Celik and A. Kara, Ann. Nucl. Energy, 37, 1705 (2010); doi:10.1016/j.anucene.2010.07.011.
- N. Damla, U. Cevik, A.I. Kobya, A. Celik, N. Celik and I. Yildirim, Radiat. Meas., 46, 701 (2011); doi:10.1016/j.radmeas.2011.06.004.
- J. Beretka and P.J. Mathew, Health Phys., 48, 87 (1985); doi:10.1097/00004032-198501000-00007.
- European Commission (EC), Radiation Protection 112. Radiological Protection Principles Concerning the Natural Radioactivity of Building Materials, Directorate-General Environment, Nuclear Safety and Civil Protection (1999).
- Organization for Economic Cooperation and Development (OECD), Exposure to Radiation from the Natural Radioactivity in Building Materials, Report by a Group of Experts of the OECD Nuclear Energy Agency (1979).
- V.R. Krieger, Betonwerk Fertigteil Tech., 47, 468 (1981).
- ICRP, Protection against Rn-222 at home and at work. Publication No. 65; Ann. ICRP 23 (2), Pergamon, Oxford (1994).
- United Nations Scientific Committee on the Effects of Atomic Radiation (UNSCEAR), Sources and Effects of Ionizing Radiation, Report of the United Nations Scientific Committee on the Effects of Atomic Radiation to the General Assembly, United Nations, New York, USA (2000).
- N. Damla, U. Cevik, A.I. Kobya, A. Celik, N. Celik and R. Van Grieken, J. Hazard. Mater., 176, 644 (2010); doi:10.1016/j.jhazmat.2009.11.080.
- United Nations Scientific Committee on the effects of atomic radiation (UNSCEAR), Ionizing Radiation: Sources and Biological Effects, United Nations, New York (1993).
- S. Turhan, J. Environ. Radioact., 99, 404 (2008); doi:10.1016/j.jenvrad.2007.11.001.
- M.O. Oresegun and A.I. Babalola, Annual Indoor Dose Burden Estimates in Dwellings Built in Nigeria with Radioactive U–Th Rich Tailings, Proceedings of an International Conference on Radiation Protection in Nuclear Energy, IAEA, Vienna, Austria 18–22 April, vol. 2, p. 159 (1988).
- P. Sorantin and F. Steger, Radiat. Prot. Dosimetry, 7, 59 (1984).
- D. Amrani and M. Tahtat, Appl. Radiat. Isot., 54, 687 (2001); doi:10.1016/S0969-8043(00)00304-3.
- S. Roy, M.S. Alam, M. Begum and B. Alam, Radiat. Prot. Dosimetry, 114, 527 (2005); doi:10.1093/rpd/nch471.
- L. Xinwei, Health Phys., 88, 84 (2005); doi:10.1097/01.HP.0000142498.08451.c8.
- M. Ngachin, M. Garavaglia, C. Giovani, M.G. Kwato Njock and A. Nourreddine, Radiat. Meas., 42, 61 (2007); doi:10.1016/j.radmeas.2006.07.007.
- O. Brígido Flores, A. Montalván Estrada, R. Rosa Suárez, J. Tomás Zerquera and A. Hernández Pérez, J. Environ. Radioact., 99, 1834 (2008); doi:10.1016/j.jenvrad.2008.08.001.
- E.M. El Afifi, M.A. Hilal, S.M. Khalifa and H.F. Aly, Radiat. Meas., 41, 627 (2006); doi:10.1016/j.radmeas.2005.09.014.
- R. Mustonen, Health Phys., 46, 1195 (1984); doi:10.1097/00004032-198406000-00003.
- C. Papastefanou, S. Stoulos and M. Manolopoulou, J. Radioanal. Nucl. Chem., 266, 367 (2005); doi:10.1007/s10967-005-0918-z.
- S. Rizzo, M. Brai, S. Basile, S. Bellia and S. Hauser, Appl. Radiat. Isot., 55, 259 (2001); doi:10.1016/S0969-8043(00)00384-5.
- R.G. Sonkawade, K. Kant, S. Muralithar, R. Kumar and R.C. Ramola, Atmos. Environ., 42, 2254 (2008); doi:10.1016/j.atmosenv.2007.11.037.
- A. Suzuki, T. Iida, J. Moriizumi and Y. Sakuma, Radiat. Prot. Dosimetry, 90, 437 (2000); doi:10.1093/oxfordjournals.rpd.a033171.
- C.S. Chong and G.U. Ahmed, Health Phys., 43, 272 (1982).
- J.G. Ackers, J.F. Den Boer, P. De Jong and R.A. Wolschrijn, Sci. Total Environ., 45, 151 (1985); doi:10.1016/0048-9697(85)90215-3.
- K. Khan and H.M. Khan, Appl. Radiat. Isot., 54, 861 (2001); doi:10.1016/S0969-8043(00)00327-4.
- S. Chinchon-Paya, B. Piedecausa, S. Hurtado, M.A. Sanjuan and S. Chinchon, Radiat. Meas., 46, 734 (2011); doi:10.1016/j.radmeas.2011.06.020.
- M. Sharaf, M. Mansy, A.A. El Sayed and E. Abbas, Radiat. Meas., 31, 491 (1999); doi:10.1016/S1350-4487(99)00206-1.
- A.O. Mustapha, D.G.S. Narayana, J.P. Patel and D. Otwoma, Radiat. Prot. Dosimetry, 71, 65 (1997); doi:10.1093/oxfordjournals.rpd.a032036.
- M.I. Chowdhury, M.N. Alam and A.K.S. Ahmed, J. Radioanal. Nucl. Chem., 231, 117 (1998); doi:10.1007/BF02388016.
- A. Malanca, V. Pessina and G. Dallara, Radiat. Prot. Dosimetry, 48, 199 (1993).
- M. Iqbal, M. Tufail and S.M. Mirza, J. Environ. Radioact., 51, 255 (2000); doi:10.1016/S0265-931X(00)00077-1.
- S. Turhan, U.N. Baykan and K. Sen, J. Radiol. Prot., 28, 83 (2008); doi:10.1088/0952-4746/28/1/005.
- L. Xinwei, Radiat. Meas., 40, 94 (2005); doi:10.1016/j.radmeas.2005.01.003.
- R.H. Higgy, M.S. El-Tahawy, A.T. Abdel-Fattah and U.A. Al-Akabawy, J. Environ. Radioact., 50, 253 (2000); doi:10.1016/S0265-931X(00)00017-5.
- J.A. Ademola and P.O. Oguneletu, J. Environ. Radioact., 81, 107 (2005); doi:10.1016/j.jenvrad.2004.12.002.
- J.A. Ademola and I.P. Farai, Radiat. Prot. Dosimetry, 121, 395 (2006); doi:10.1093/rpd/ncl052.
- N. Ibrahim, J. Environ. Radioact., 43, 255 (1999); doi:10.1016/S0265-931X(98)00033-2.
References
E. Yilmaz, H. Baltas, E. Kiris, İ. Ustabas, U. Cevik and A.M. El-Khayatt, Ann. Nucl. Energy, 38, 2204 (2011); doi:10.1016/j.anucene.2011.06.011.
V. Kumar, T.V. Ramachandran and R. Prasad, Appl. Radiat. Isot., 51, 93 (1999); doi:10.1016/S0969-8043(98)00154-7.
O. Baykara, Ş. Karatepe and M. Doğru, Radiat. Meas., 46, 153 (2011); doi:10.1016/j.radmeas.2010.08.010.
N. Kovler, G. Haquin, V. Manasherov, E. Ne’eman and N. Lavi, Build. Environ., 37, 531 (2002); doi:10.1016/S0360-1323(01)00048-8.
S. Stoulos, M. Manolopoulou and C. Papastefanou, J. Environ. Radioact., 69, 225 (2003); doi:10.1016/S0265-931X(03)00081-X.
B. Mavi and I. Akkurt, Radiat. Phys. Chem., 79, 933 (2010); doi:10.1016/j.radphyschem.2010.03.019.
H. Papaefthymiou and O. Gouseti, Radiat. Meas., 43, 1453 (2008); doi:10.1016/j.radmeas.2008.03.032.
R. Hewamanna, C.S. Sumithrarachchi, P. Mahawatte, H.L.C. Nanayakkara and H.C. Ratnayake, Appl. Radiat. Isot., 54, 365 (2001); doi:10.1016/S0969-8043(00)00107-X.
N.P. Petropoulos, M.J. Anagnostakis and S.E. Simopoulos, J. Environ. Radioact., 61, 257 (2002); doi:10.1016/S0265-931X(01)00132-1.
X. Lu, G. Yang and C. Ren, Radiat. Phys. Chem., 81, 780 (2012); doi:10.1016/j.radphyschem.2012.02.043.
U. Cevik, N. Damla, A.I. Kobya, A. Celik and A. Kara, Ann. Nucl. Energy, 37, 1705 (2010); doi:10.1016/j.anucene.2010.07.011.
N. Damla, U. Cevik, A.I. Kobya, A. Celik, N. Celik and I. Yildirim, Radiat. Meas., 46, 701 (2011); doi:10.1016/j.radmeas.2011.06.004.
J. Beretka and P.J. Mathew, Health Phys., 48, 87 (1985); doi:10.1097/00004032-198501000-00007.
European Commission (EC), Radiation Protection 112. Radiological Protection Principles Concerning the Natural Radioactivity of Building Materials, Directorate-General Environment, Nuclear Safety and Civil Protection (1999).
Organization for Economic Cooperation and Development (OECD), Exposure to Radiation from the Natural Radioactivity in Building Materials, Report by a Group of Experts of the OECD Nuclear Energy Agency (1979).
V.R. Krieger, Betonwerk Fertigteil Tech., 47, 468 (1981).
ICRP, Protection against Rn-222 at home and at work. Publication No. 65; Ann. ICRP 23 (2), Pergamon, Oxford (1994).
United Nations Scientific Committee on the Effects of Atomic Radiation (UNSCEAR), Sources and Effects of Ionizing Radiation, Report of the United Nations Scientific Committee on the Effects of Atomic Radiation to the General Assembly, United Nations, New York, USA (2000).
N. Damla, U. Cevik, A.I. Kobya, A. Celik, N. Celik and R. Van Grieken, J. Hazard. Mater., 176, 644 (2010); doi:10.1016/j.jhazmat.2009.11.080.
United Nations Scientific Committee on the effects of atomic radiation (UNSCEAR), Ionizing Radiation: Sources and Biological Effects, United Nations, New York (1993).
S. Turhan, J. Environ. Radioact., 99, 404 (2008); doi:10.1016/j.jenvrad.2007.11.001.
M.O. Oresegun and A.I. Babalola, Annual Indoor Dose Burden Estimates in Dwellings Built in Nigeria with Radioactive U–Th Rich Tailings, Proceedings of an International Conference on Radiation Protection in Nuclear Energy, IAEA, Vienna, Austria 18–22 April, vol. 2, p. 159 (1988).
P. Sorantin and F. Steger, Radiat. Prot. Dosimetry, 7, 59 (1984).
D. Amrani and M. Tahtat, Appl. Radiat. Isot., 54, 687 (2001); doi:10.1016/S0969-8043(00)00304-3.
S. Roy, M.S. Alam, M. Begum and B. Alam, Radiat. Prot. Dosimetry, 114, 527 (2005); doi:10.1093/rpd/nch471.
L. Xinwei, Health Phys., 88, 84 (2005); doi:10.1097/01.HP.0000142498.08451.c8.
M. Ngachin, M. Garavaglia, C. Giovani, M.G. Kwato Njock and A. Nourreddine, Radiat. Meas., 42, 61 (2007); doi:10.1016/j.radmeas.2006.07.007.
O. Brígido Flores, A. Montalván Estrada, R. Rosa Suárez, J. Tomás Zerquera and A. Hernández Pérez, J. Environ. Radioact., 99, 1834 (2008); doi:10.1016/j.jenvrad.2008.08.001.
E.M. El Afifi, M.A. Hilal, S.M. Khalifa and H.F. Aly, Radiat. Meas., 41, 627 (2006); doi:10.1016/j.radmeas.2005.09.014.
R. Mustonen, Health Phys., 46, 1195 (1984); doi:10.1097/00004032-198406000-00003.
C. Papastefanou, S. Stoulos and M. Manolopoulou, J. Radioanal. Nucl. Chem., 266, 367 (2005); doi:10.1007/s10967-005-0918-z.
S. Rizzo, M. Brai, S. Basile, S. Bellia and S. Hauser, Appl. Radiat. Isot., 55, 259 (2001); doi:10.1016/S0969-8043(00)00384-5.
R.G. Sonkawade, K. Kant, S. Muralithar, R. Kumar and R.C. Ramola, Atmos. Environ., 42, 2254 (2008); doi:10.1016/j.atmosenv.2007.11.037.
A. Suzuki, T. Iida, J. Moriizumi and Y. Sakuma, Radiat. Prot. Dosimetry, 90, 437 (2000); doi:10.1093/oxfordjournals.rpd.a033171.
C.S. Chong and G.U. Ahmed, Health Phys., 43, 272 (1982).
J.G. Ackers, J.F. Den Boer, P. De Jong and R.A. Wolschrijn, Sci. Total Environ., 45, 151 (1985); doi:10.1016/0048-9697(85)90215-3.
K. Khan and H.M. Khan, Appl. Radiat. Isot., 54, 861 (2001); doi:10.1016/S0969-8043(00)00327-4.
S. Chinchon-Paya, B. Piedecausa, S. Hurtado, M.A. Sanjuan and S. Chinchon, Radiat. Meas., 46, 734 (2011); doi:10.1016/j.radmeas.2011.06.020.
M. Sharaf, M. Mansy, A.A. El Sayed and E. Abbas, Radiat. Meas., 31, 491 (1999); doi:10.1016/S1350-4487(99)00206-1.
A.O. Mustapha, D.G.S. Narayana, J.P. Patel and D. Otwoma, Radiat. Prot. Dosimetry, 71, 65 (1997); doi:10.1093/oxfordjournals.rpd.a032036.
M.I. Chowdhury, M.N. Alam and A.K.S. Ahmed, J. Radioanal. Nucl. Chem., 231, 117 (1998); doi:10.1007/BF02388016.
A. Malanca, V. Pessina and G. Dallara, Radiat. Prot. Dosimetry, 48, 199 (1993).
M. Iqbal, M. Tufail and S.M. Mirza, J. Environ. Radioact., 51, 255 (2000); doi:10.1016/S0265-931X(00)00077-1.
S. Turhan, U.N. Baykan and K. Sen, J. Radiol. Prot., 28, 83 (2008); doi:10.1088/0952-4746/28/1/005.
L. Xinwei, Radiat. Meas., 40, 94 (2005); doi:10.1016/j.radmeas.2005.01.003.
R.H. Higgy, M.S. El-Tahawy, A.T. Abdel-Fattah and U.A. Al-Akabawy, J. Environ. Radioact., 50, 253 (2000); doi:10.1016/S0265-931X(00)00017-5.
J.A. Ademola and P.O. Oguneletu, J. Environ. Radioact., 81, 107 (2005); doi:10.1016/j.jenvrad.2004.12.002.
J.A. Ademola and I.P. Farai, Radiat. Prot. Dosimetry, 121, 395 (2006); doi:10.1093/rpd/ncl052.
N. Ibrahim, J. Environ. Radioact., 43, 255 (1999); doi:10.1016/S0265-931X(98)00033-2.