Bio-Oil Model Compounds Upgrading Under CO Atmosphere

Qingli Xu1; Weidi Dai1; Jianchun Jiang1; Yongjie Yan2

doi:10.14233/ajchem.2014.15415

Issue

Vol. 26 No. 2 (2014): Vol 26 Issue 2

Issue Published : January 15, 2014

This work is licensed under a Creative Commons Attribution 4.0 International License.

Bio-Oil Model Compounds Upgrading Under CO Atmosphere

https://doi.org/10.14233/ajchem.2014.15415

Qingli Xu1

1Jiangsu Key Laboratory for Biomass Energy and Material, Nanjing 210042, Jiangsu Province, P.R. China 2Key Laboratory of Coal Gasification and Energy Chemical Engineering of Ministry of Education; Research Center for Biomass Energy, East China University of Science and Technology, Shanghai 200237, P.R. China *Corresponding author: E-mail: xuqingli2001@163.com

Weidi Dai1

Jianchun Jiang1

Yongjie Yan2

Asian Journal of Chemistry, Vol. 26 No. 2 (2014): Vol 26 Issue 2
Article Published : January 16, 2014

Abstract

The bio-oil model upgrading was studied over a series of catalysts in the CO/H₂O system. The impregnation method was superior to the dry mix method. 6 % of Ni impregnating in B206 catalyst is the optimum bi-functional catalyst. The optimum catalyst showed the highest activity for deoxygenation in the CO/H₂O system, the deoxygenation rate was up to 92 % and the dehydration rate was 89 % in a certain conditions after upgrading.

Keywords

Bio-oil Model Deoxygenation Upgrading Bi-functional catalyst.

Xu1, Q., Dai1, W., Jiang1, J., & Yan2, Y. (2014). Bio-Oil Model Compounds Upgrading Under CO Atmosphere. Asian Journal of Chemistry, 26(2), 403–406. https://doi.org/10.14233/ajchem.2014.15415

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References

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References

B. Acharya, A. Dutta and P. Basu, Int. J. Hydrogen Energy, 35, 1582 (2010); doi:10.1016/j.ijhydene.2009.11.109.

S. Luo, C. Yi and Y. Zhou, Renew. Energy, 36, 3332 (2011); doi:10.1016/j.renene.2011.05.006.

Y. Sun and J. Cheng, Bioresour. Technol., 83, 1 (2002); doi:10.1016/S0960-8524(01)00212-7.

C.N. Hamelinck, G. Hooijdonk and A.P.C. Faaij, Biomass Bioenergy, 28, 384 (2005); doi:10.1016/j.biombioe.2004.09.002.

M.R. Ladisch and J.A. Svarczkopf, Bioresour. Technol., 36, 83 (1991); doi:10.1016/0960-8524(91)90102-P.

J. Lédé, F. Broust, F.T. Ndiaye and M. Ferrer, Fuel, 86, 1800 (2007); doi:10.1016/j.fuel.2006.12.024.

J. Zheng, J. Anal. Appl. Pyrol., 80, 30 (2007); doi:10.1016/j.jaap.2006.12.030.

D.S. Scott and J. Piskorz, Can. J. Chem. Eng., 60, 666 (1982); doi:10.1002/cjce.5450600514.

B. Krieger-Brockett, Res. Chem. Intermed., 20, 39 (1994); doi:10.1163/156856794X00054.

M. Garcìa-Pérez, A. Chaala, H. Pakdel, D. Kretschmer and C. Roy, J. Anal. Appl. Pyrolysis, 78, 104 (2007); doi:10.1016/j.jaap.2006.05.003.

J. Diebold and J. Scahill, ACS Preprints (Div. Fuel Chem.), 32, 21 (1987).

B.M. Wagenaar, W. Prins and W.P.M. Vanswaaij, Chem. Eng. Sci., 49, 5109 (1994); doi:10.1016/0009-2509(94)00392-0.

D. Chiaramonti, M. Bonini, E. Fratini, G. Tondi, K. Gartner, A.V. Bridgwater, H.P. Grimm, I. Soldaini, A. Webster and P. Baglioni, Biomass Bioenergy, 25, 85 (2003); doi:10.1016/S0961-9534(02)00183-6.

D. Chiaramonti, M. Bonini, E. Fratini, G. Tondi, K. Gartner, A.V. Bridgwater, H.P. Grimm, I. Soldaini, A. Webster and P. Baglioni, Biomass Bioenergy, 25, 101 (2003); doi:10.1016/S0961-9534(02)00184-8.

S. Wang, Y. Gu, Q. Liu, Y. Yao, Z. Guo, Z. Luo and K. Cen, Fuel Process. Technol., 90, 738 (2009); doi:10.1016/j.fuproc.2009.02.005.

J.N. Murwanashyaka, H. Pakdel and C. Roy, Sep. Purif. Technol., 24, 155 (2001); doi:10.1016/S1383-5866(00)00225-2.

C. Amen-Chen, H. Pakdel and C. Roy, Biomass Bioenergy, 13, 25 (1997); doi:10.1016/S0961-9534(97)00021-4.

S. Panigrahi, A.K. Dalai, S.T. Chaudhari and N.N. Bakhshi, Energy Fuels, 17, 637 (2003); doi:10.1021/ef020073z.

N. Gao, A. Li and C. Quan, Bioresour. Technol., 100, 4271 (2009); doi:10.1016/j.biortech.2009.03.045.

Q. Xu, P. Lan, B. Zhang, Z. Ren and Y. Yan, Energy Fuels, 24, 6456 (2010); doi:10.1021/ef1010995.

R.K. Sharma and N.N. Bakhshi, Bioresour. Technol., 45, 195 (1993); doi:10.1016/0960-8524(93)90112-O.

C.A. Fisk, T. Morgan, Y. Ji, M. Crocker, C. Crofcheck and S.A. Lewis, Appl. Catal. A Gen., 358, 150 (2009); doi:10.1016/j.apcata.2009.02.006.

S. Miao and B.H. Shanks, Appl. Catal. A Gen., 359, 113 (2009); doi:10.1016/j.apcata.2009.02.029.

K. Sipila, E. Kuoppala, L. Fagernas and A. Oasmaa, Biomass Bioenergy, 14, 103 (1998); doi:10.1016/S0961-9534(97)10024-1.

Q. Xu, H. Zhang, S. Li, W. Dai, J. Jiang and Y. Yan, Asian J. Chem., 25, 3789 (2013).

Issue

Vol. 26 No. 2 (2014): Vol 26 Issue 2

Bio-Oil Model Compounds Upgrading Under CO Atmosphere

Abstract

Keywords

Full Article

Download Citation

References

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