Copyright (c) 2013 AJC
This work is licensed under a Creative Commons Attribution 4.0 International License.
Wastewater Treatment by CNT/TiO2 Composites Prepared from Multi-Walled Carbon Nanotubes with Different Organo-Titanium Precursors
Corresponding Author(s) : Won-Chun Oh
Asian Journal of Chemistry,
Vol. 25 No. 6 (2013): Vol 25 Issue 6
Abstract
We prepared CNT/TiO2 composites by using pre-oxidized multi-walled carbon nanotubes with different titanium alkoxide precursors in benzene solvent. The composites were comprehensively characterized by Brauer-Emett-Teller surface area, transmission electron microscopy, X-ray diffraction and energy dispersive X-ray analysis. Furthermore, we used the prepared CNT/TiO2 composites to decompose the piggery waste under UV irradiation. The decomposition effect was analyzed by using the chemical oxygen demand method, FT-IR spectra, absorbance and total organic carbon. According to the results, after UV irradiation for 300 min, the chemical oxygen demand value was decreased 50 % and the organic compounds in piggery waste were degraded to other matters.
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- E. Sanchez, P. Weiland and L. Travieso, Bioresour. Technol., 47, 173 (1994).
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- A. Jitianu, T. Cacciaguerra, R. Benoit, S. Delpeux, F. Beguin and S. Bonnamy, Carbon, 42, 1147 (2004).
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- W.C. Oh and M.L. Chen, Bull. Korean Chem. Soc., 29, 159 (2008).
- H.S. Yoon, S.K. Ryu, W.C. Oh and F.J. Zhang, Asian J. Chem., 24, 621 (2012).
- M.L. Chen, F.J. Zhang and W.C. Oh, J. Korean Ceramic Soc., 45, 651 (2008).
- M.L Chen, F.J. Zhang and W.C. Oh, Bull. Mater. Sci., 34, 835 (2011).
- F.J. Zhang and W.C. Oh, J. Ind. Eng. Chem., 31, 7 (2010).
- W.C. Oh and W.B. Ko, J. Ind. Eng. Chem., 12, 373 (2006).
- K. Hernadi, E. Ljubovic, J.W. Seo and L. Forro,Acta Mater.,51, 1447 (2003).
- W. Wang, P. Serp, P. Kalck and J.L. Faria, Appl. Catal. B, 56, 305 (2005).
- J. Sun, L. Gao and M. Iwasa, Chem. Comm., 7, 832 (2004).
- K. Zhang, F.J. Zhang, M.L. Chen and W.C. Oh, Ultrason. Sonochem., 18, 765 (2011).
- K. Zhang, J.G. Choi and W.C. Oh, Asian J. Chem., 23, 356 (2011).
- P.A. Bianco, M. Vincenti, A. Banciotto and E. Pramauro, Appl. Catal. B: Environ., 22, 149 (1999).
- C.S. Lua, C.C. Chen, F.D. Mai and H.K. Li, J. Hazard. Mater., 165, 306 (2009)
References
E. Sanchez, P. Weiland and L. Travieso, Bioresour. Technol., 47, 173 (1994).
C.E. Domini, M. Hidalgo, F. Marken and A. Canals, Anal. Chim. Acta, 561, 210 (2006).
B.X. Li, Z.J. Zhang, J. Wang and C.L. Xu, Talanta, 61, 651 (2003).
R. Devi and R.P. Dahiya, Water Air Soil Pollut., 174, 33 (2006).
B. Mounir, M.N. Pons, O. Zahraa, A. Yaacoubi and A. Benhammou, J. Hazard. Mater., 148, 513 (2007).
Z. Zainal, C.Y. Lee, M.Z. Hussein, A. Kassein and N.A. Yusof, J. Hazard. Mater., 146, 73 (2007).
P. Saritha, C. Aparna, V. Himabindu and Y. Anjaneyulu, J. Hazard. Mater., 149, 609 (2007).
M.G. Neelavannan, M. Revathi and C.A. Basha, J. Hazard. Mater., 149, 371 (2007).
O. Gimeno, M. Carbajo, F.J. Beltran and F.J. Rivas, J. Hazard. Mater., B119, 99 (2005).
J.P. Salvetat-Delmontte and A. Rubio, Carbon, 40, 1729 (2000).
T. Saito, K. Matsushige and K. Tanaka, Physica B, 323, 280 (2002).
A. Jitianu, T. Cacciaguerra, R. Benoit, S. Delpeux, F. Beguin and S. Bonnamy, Carbon, 42, 1147 (2004).
W.D. Wang, P. Serp, P. Kalck and J.L. Faria, J. Mol. Catal. A, 235, 194 (2005).
W.C. Oh and M.L. Chen, Bull. Korean Chem. Soc., 29, 159 (2008).
H.S. Yoon, S.K. Ryu, W.C. Oh and F.J. Zhang, Asian J. Chem., 24, 621 (2012).
M.L. Chen, F.J. Zhang and W.C. Oh, J. Korean Ceramic Soc., 45, 651 (2008).
M.L Chen, F.J. Zhang and W.C. Oh, Bull. Mater. Sci., 34, 835 (2011).
F.J. Zhang and W.C. Oh, J. Ind. Eng. Chem., 31, 7 (2010).
W.C. Oh and W.B. Ko, J. Ind. Eng. Chem., 12, 373 (2006).
K. Hernadi, E. Ljubovic, J.W. Seo and L. Forro,Acta Mater.,51, 1447 (2003).
W. Wang, P. Serp, P. Kalck and J.L. Faria, Appl. Catal. B, 56, 305 (2005).
J. Sun, L. Gao and M. Iwasa, Chem. Comm., 7, 832 (2004).
K. Zhang, F.J. Zhang, M.L. Chen and W.C. Oh, Ultrason. Sonochem., 18, 765 (2011).
K. Zhang, J.G. Choi and W.C. Oh, Asian J. Chem., 23, 356 (2011).
P.A. Bianco, M. Vincenti, A. Banciotto and E. Pramauro, Appl. Catal. B: Environ., 22, 149 (1999).
C.S. Lua, C.C. Chen, F.D. Mai and H.K. Li, J. Hazard. Mater., 165, 306 (2009)